An analysis method proposed by Huang is improved and used to dissect the radiative forcing in the instantaneous quadrupling CO2 experiment from phase 5 of the Coupled Model Intercomparison Project (CMIP5). Multiple validation tests show that the errors in the forcing estimates are generally within 10%. The results show that quadrupling CO2, on average, induces a global-mean all-sky instantaneous top-of-the-atmosphere forcing of 5.4 W m−2, which is amended by a stratospheric adjustment of 1.9 W m−2 and a tropospheric adjustment of −0.1 W m−2. The resulting fully adjusted radiative forcing has an ensemble mean of 7.2 W m−2 and a substantial intermodel spread (maximum–minimum) of 2.4 W m−2, which results from all the forcing components, especially the instantaneous forcing and tropospheric adjustment. The fidelity of the linear decomposition of the overall radiation variation is improved when forcing is explicitly estimated for each model. A significant contribution by forcing uncertainty to the intermodel spread of the surface temperature projection is verified. The results reaffirm the importance of evaluating the radiative forcing components in climate feedback analyses.